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VIENNA — Nine days into marathon nuclear talks, U.S. Secretary of State John Kerry on Sunday said the diplomatic efforts “could go either way,” cutting off all potential pathways for an Iranian atomic bomb or ending without an agreement that American officials have sometimes described as the only alternative to war.

“I want to be absolutely clear with everybody: We are not yet where we need to be on several of the most critical issues,” Kerry told reporters outside the 19th-century Viennese palace that has hosted the negotiations.

World powers and Iran are hoping to clinch a deal by Tuesday, setting a decade of restrictions on Iran’s nuclear program and granting Iran significant relief from international sanctions. Kerry met for 3½ hours on Sunday with Iranian Foreign Minister Mohammad Javad Zarif, as top diplomats from the five other negotiating countries planned to return to Austria’s capital later in the evening.

The talks had appeared to be moving forward. On Saturday, diplomats reported tentative agreement on the speed and scope of sanctions relief for Iran in the accord, even as issues such as inspection guidelines and limits on Iran’s nuclear research and development remained contentious.

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